Interview with Robert V. Pound done in 5 sessions. Topics discussed include: Henry Torrey; Pound's physics degree earned at University of Buffalo, where his father was a physics professor; I. I. Rabi's, Jerold Zacharias' and A. G. Hill's roles as superiors and mentors in Radiation Laboratory days and in early nuclear magnetic resonance (NMR) work; his interactions with Otto Frisch, Lise Meitner, Victor Weisskopf, John Van Vleck, George Pake; his start in amateur radio; his professorship at Harvard and his objection to core curriculum; his Submarine Signal Company sonar and radar work; the Tizard mission; E. G. Bowen; his time as chair of Harvard physics department; molecular beams and magnetic resonance; C. J. Gorter's summer at Harvard; Alfred Loomis; Erwin Hahn and spin echoes; signal to noise work at Massachusetts Institute of Technology (MIT); Bell Laboratories; NMR amplifier; gravitational redshift experiments, 1960-1964; use of cyclotrons to make radioactive sources; Joe Snyder, Robert Dickey; competition with the Harwell Group on gravitational redshift; George Gamow; Ed Condon; year at Oxford; Olah Bohr; John Tate; Francis Bitter; and Luis Alvarez; classical versus quantum mechanics; C. P. Snow and Lord Charwell.